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Shimalactone Biosynthesis Involves Spontaneous Double Bicyclo-Ring Formation with 8π-6π Electrocyclization.
Fujii I, Hashimoto M, Konishi K, Unezawa A, Sakuraba H, Suzuki K, Tsushima H, Iwasaki M, Yoshida S, Kudo A, Fujita R, Hichiwa A, Saito K, Asano T, Ishikawa J, Wakana D, Goda Y, Watanabe A, Watanabe M, Masumoto Y, Kanazawa J, Sato H, Uchiyama M. Fujii I, et al. Among authors: goda y. Angew Chem Int Ed Engl. 2020 May 25;59(22):8464-8470. doi: 10.1002/anie.202001024. Epub 2020 Mar 20. Angew Chem Int Ed Engl. 2020. PMID: 32129542
Functional expression of a highly-reducing polyketide synthase of Emericella variecolor IFM42010, an asteltoxin-producing strain, resulted in production of two polyenoic β-ketolactones with opposite stereochemistry.
Hashimoto M, Ichijo H, Fujiwara K, Sugasawa H, Abo S, Matsudo K, Uchiyama N, Goda Y, Fujii I. Hashimoto M, et al. Among authors: goda y. Bioorg Med Chem Lett. 2019 Dec 15;29(24):126686. doi: 10.1016/j.bmcl.2019.126686. Epub 2019 Oct 14. Bioorg Med Chem Lett. 2019. PMID: 31678008
504 results