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Understanding Synergistic Catalysis on Cu-Se Dual Atom Sites via Operando X-ray Absorption Spectroscopy in Oxygen Reduction Reaction.
Sun Z, Zhang H, Cao L, Liu X, Wu D, Shen X, Zhang X, Chen Z, Ru S, Zhu X, Xia Z, Luo Q, Xu F, Yao T. Sun Z, et al. Angew Chem Int Ed Engl. 2023 Mar 20;62(13):e202217719. doi: 10.1002/anie.202217719. Epub 2023 Feb 10. Angew Chem Int Ed Engl. 2023. PMID: 36692894
The heteroatom Se modulator can efficiently polarize the charge distribution around symmetrical Cu-N(4) moieties, and serve as synergistic site to facilitate the second oxygen reduction step simultaneously, in which the key OOH*-(Cu(1) -N(4) ) transforms to O*-(Se(1) -C(2) …
The heteroatom Se modulator can efficiently polarize the charge distribution around symmetrical Cu-N(4) moieties, and serve as synergistic s …