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Switching the redox mechanism: models for proton-coupled electron transfer from tyrosine and tryptophan.
Sjödin M, Styring S, Wolpher H, Xu Y, Sun L, Hammarström L. Sjödin M, et al. J Am Chem Soc. 2005 Mar 23;127(11):3855-63. doi: 10.1021/ja044395o. J Am Chem Soc. 2005. PMID: 15771521
By altering the solution pH, the strength of the Ru(III) oxidant, or the identity of the amino acid, we could induce a switch between the two mechanisms and obtain quantitative data for the parameters that control which one will dominate. The characteristic pH-dependence of the C …
By altering the solution pH, the strength of the Ru(III) oxidant, or the identity of the amino acid, we could induce a switch between the tw …
Kinetic effects of hydrogen bonds on proton-coupled electron transfer from phenols.
Sjödin M, Irebo T, Utas JE, Lind J, Merényi G, Akermark B, Hammarström L. Sjödin M, et al. J Am Chem Soc. 2006 Oct 11;128(40):13076-83. doi: 10.1021/ja063264f. J Am Chem Soc. 2006. PMID: 17017787
Without internal hydrogen bonds the concerted mechanism gave a characteristic pH-dependent rate for the phenol form that followed a Marcus free energy dependence, first reported for an intramolecular PCET in Sjodin, M. et al. J. Am. Chem. Soc. 2000, 122, 3932-3962 a …
Without internal hydrogen bonds the concerted mechanism gave a characteristic pH-dependent rate for the phenol form that followed a Marcus f …
An All-Organic Proton Battery.
Emanuelsson R, Sterby M, Strømme M, Sjödin M. Emanuelsson R, et al. Among authors: sjodin m. J Am Chem Soc. 2017 Apr 5;139(13):4828-4834. doi: 10.1021/jacs.7b00159. Epub 2017 Mar 28. J Am Chem Soc. 2017. PMID: 28293954
73 results