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Constructing a Stable Interface Layer by Tailoring Solvation Chemistry in Carbonate Electrolytes for High-Performance Lithium-Metal Batteries.
Piao Z, Xiao P, Luo R, Ma J, Gao R, Li C, Tan J, Yu K, Zhou G, Cheng HM. Piao Z, et al. Among authors: li c. Adv Mater. 2022 Feb;34(8):e2108400. doi: 10.1002/adma.202108400. Epub 2022 Jan 14. Adv Mater. 2022. PMID: 34859925
By introducing lithium nitrate additive and a small amount of tetramethylurea as a multifunctional cosolvent to a commercial carbonate electrolyte, NO(3) (-) , which is usually insoluble, can be introduced into the solvation structure of Li(+) to form a conductive and stab …
By introducing lithium nitrate additive and a small amount of tetramethylurea as a multifunctional cosolvent to a commercial carbonate elect …
A 3D Framework with Li3 N-Li2 S Solid Electrolyte Interphase and Fast Ion Transfer Channels for a Stabilized Lithium-Metal Anode.
Ni S, Zhang M, Li C, Gao R, Sheng J, Wu X, Zhou G. Ni S, et al. Among authors: li c. Adv Mater. 2023 Feb;35(8):e2209028. doi: 10.1002/adma.202209028. Epub 2022 Dec 23. Adv Mater. 2023. PMID: 36482265
The Li-metal anode has been recognized as the most promising anode for its high theoretical capacity and low reduction potential. However, the major drawbacks of Li metal, such as high reactivity and large volume expansion, can lead to dendrite growth and solid elec …
The Li-metal anode has been recognized as the most promising anode for its high theoretical capacity and low reduction potential. How …
Stable Operation of Lithium Metal Batteries with Aggressive Cathode Chemistries at 4.9 V.
Piao Z, Ren HR, Lu G, Jia K, Tan J, Wu X, Zhuang Z, Han Z, Li C, Gao R, Tao X, Zhou G, Cheng HM. Piao Z, et al. Among authors: li c. Angew Chem Int Ed Engl. 2023 Apr 3;62(15):e202300966. doi: 10.1002/anie.202300966. Epub 2023 Mar 2. Angew Chem Int Ed Engl. 2023. PMID: 36788164
Meanwhile, robust and elastic B and F-rich interphases are formed on both electrodes. Such optimization enables Li||LiNi(0.5) Mn(1.5) O(4) cells (90.2 % retention after 400 cycles) and Li||LiNi(0.6) Co(0.2) Mn(0.2) O(2) (NCM622) cells (74.0 % retention after 200 cyc …
Meanwhile, robust and elastic B and F-rich interphases are formed on both electrodes. Such optimization enables Li||LiNi(0.5) Mn(1.5) …
Uncoordinated chemistry enables highly conductive and stable electrolyte/filler interfaces for solid-state lithium-sulfur batteries.
Zhu Y, Zhang Q, Zheng Y, Li G, Gao R, Piao Z, Luo D, Gao RH, Zhang M, Xiao X, Li C, Lao Z, Wang J, Chen Z, Zhou G. Zhu Y, et al. Among authors: li c, li g. Proc Natl Acad Sci U S A. 2023 Apr 11;120(15):e2300197120. doi: 10.1073/pnas.2300197120. Epub 2023 Apr 5. Proc Natl Acad Sci U S A. 2023. PMID: 37018192 Free PMC article.
Moreover, the as-exposed Lewis-acid metal centers in UCPBA efficiently attract the Lewis-base anions of Li salts, which facilitates the Li(+) disassociation and enhances its transference number (t(Li)(+)). Attributed to these superiorities, the obtained CPEs …
Moreover, the as-exposed Lewis-acid metal centers in UCPBA efficiently attract the Lewis-base anions of Li salts, which facilitates t …
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