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Selective CO2 Photoreduction Enabled by Water-stable Cu-based Metal-organic Framework Nanoribbons.
Zhao Y, Chen R, Luo J, Zhu J, Wu Y, Qiao P, Yan W, Pan Y, Zhu J, Zu X, Sun Y. Zhao Y, et al. Chemphyschem. 2024 Mar 1;25(5):e202300368. doi: 10.1002/cphc.202300368. Epub 2024 Jan 26. Chemphyschem. 2024. PMID: 38193665
In situ Fourier-transform infrared spectra and Gibbs free energy calculations unravel the formation of the key intermediate COOH* and CO* is an exothermic and spontaneous process, whereas the competitive hydrogen evolution reaction is endothermic and non-spontaneous, which …
In situ Fourier-transform infrared spectra and Gibbs free energy calculations unravel the formation of the key intermediate COOH* and …
Atom-Economical Synthesis of Dimethyl Carbonate from CO2 : Engineering Reactive Frustrated Lewis Pairs on Ceria with Vacancy Clusters.
Li L, Liu W, Chen R, Shang S, Zhang X, Wang H, Zhang H, Ye B, Xie Y. Li L, et al. Angew Chem Int Ed Engl. 2022 Dec 19;61(51):e202214490. doi: 10.1002/anie.202214490. Epub 2022 Nov 22. Angew Chem Int Ed Engl. 2022. PMID: 36307955
By taking CeO(2) as a model system, we illustrate that FLP sites can efficiently accelerate the coupling and conversion of key intermediates. As demonstrated, CeO(2) with rich FLP sites shows improved reaction activity and achieves a high yield of DMC up to 15.3 mmol g(-1) …
By taking CeO(2) as a model system, we illustrate that FLP sites can efficiently accelerate the coupling and conversion of key interm …