Spatiotemporal empirical analysis of particulate matter PM2.5 pollution and air quality index (AQI) trends in Africa using MERRA-2 reanalysis datasets (1980-2021)

Sci Total Environ. 2024 Feb 20:912:169027. doi: 10.1016/j.scitotenv.2023.169027. Epub 2023 Dec 8.

Abstract

In this study, the spatial-temporal trends of PM2.5 pollution were analyzed for subregions in Africa and the entire continent from 1980 to 2021. The distributions and trends of PM2.5 were derived from the monthly concentrations of the aerosol species from MERRA-2 reanalysis datasets comprising of sulphates (SO4), organic carbon (OC), black carbon (BC), Dust2.5 and Sea Salt (SS2.5). The resulting PM2.5 trends were compared with the climate factors, socio-economic indicators, and terrain characteristics. Using the Mann-Kendall (M-K) test, the continent and its subregions showed positive trends in PM2.5 concentrations, except for western and central Africa which exhibited marginal negative trends. The M-K trends also determined Dust2.5 as the dominant contributing aerosol factor responsible for the high PM2.5 concentrations in the northern, western and central regions of Africa, while SO4 and OC were respectively the most significant contributors to PM2.5 in the eastern and southern Africa regions. For the climate factors, the PM2.5 trends were determined to be positively correlated with the wind speed trends, while precipitation and temperature trends exhibited low and sometimes negative correlations with PM2.5. Socio-economically, highly populated, and bare/sparse vegetated areas showed higher PM2.5 concentrations, while vegetated areas tended to have lower PM2.5 concentrations. Topographically, low laying regions were observed to retain the deposited PM2.5 especially in the northern and western regions of Africa. The Air Quality Index (AQI) results showed that 94 % of the continent had an average PM2.5 of 12-35 μg/m3 hence classified as "Moderate" AQI, and the rest of the continent's PM2.5 levels was between 35 and 55 μg/m3 implying AQI classification of "Unhealthy for Sensitive People". Northern and western Africa regions had the highest AQI, while southern Africa had the lowest AQI. The approach and findings in this study can be used to complement the evaluation and management of air quality in Africa.

Keywords: Air quality index; MERRA-2; Meteorological factors; PM(2.5); Pollution in Africa; Socio-economic indicators.