Spectral mapping of the third-order optical nonlinearity of glass-metal nanocomposites

Opt Express. 2009 Sep 14;17(19):17170-8. doi: 10.1364/OE.17.017170.

Abstract

By tuning wavelengths of the femtosecond pump and probe pulses we mapped the nonlinear absorption of copper-glass nanocomposites within 520-620 nm range. At the pump intensity of 3 GW/cm(2), the induced transmission rise was as high as 20%. The imaginary part of the third-order optical susceptibility of the nanocomposites as a function of the probe wavelength reproduced well the spectral profile of the surface plasmon resonance in copper. In contrast, the imaginary part of the third-order optical susceptibility as a function of the pump wavelength did not reproduce the plasmon profile being wider than the latter.

Publication types

  • Research Support, Non-U.S. Gov't