This paper proposes a simple, stable, sensitive, and angle-dependent localized surface plasmon resonance (LSPR) sensing structure based on multi-mode optical fiber. We adopted the template transfer method to integrate a nanohole array onto a fiber tip with beveled angle. Experimental results indicated that beveled angle structured probe sensor outperform the flat optical fiber tip structured LSPR sensor in our experiment. We tested the sensitivity and the figure of merit (FOM) of the probe beveled angle from 5°-22°, with refractive index ranging from 1.333-1.385, to find that sensitivity and FOM were optimal at fiber tip bevel angle of 7°, reaching 487 nm/RIU and 29 respectively.