A study of helium-3 nuclear magnetic relaxation mechanism in contact with 20 nm DyF3 nanoparticles

J Magn Reson. 2024 May:362:107672. doi: 10.1016/j.jmr.2024.107672. Epub 2024 Apr 22.

Abstract

The spin kinetics of adsorbed and liquid 3He in contact with a mixture of LaF3 (99.67 %) and DyF3 (0.33 %) 20 nm powders at temperatures of 1.5-4.2 K in magnetic fields up to 505mT was studied by pulsed nuclear magnetic resonance (NMR). Two-component of nuclear magnetic relaxation was observed in the experiment and theoretical relaxation model was proposed. The possible explanation of this phenomena can be carried out by a model that consider the exchange of magnetization of helium-3 nuclei located in the adsorbed layer and in the bulk of the liquid. The proposed relaxation model can be applied to other systems with the strong influence of adsorbed layer.

Keywords: Helium-3; Nanoparticles; Nuclear magnetic resonance; Relaxation mechanism.