Interannual variations in ozone pollution with a dipole structure over Eastern China associated with springtime thermal forcing over the Tibetan Plateau

Qingjian Yang; Tianliang Zhao; Yongqing Bai; Jing Wei; Xiaoyun Sun; Zhijie Tian; Jun Hu; Xiaodan Ma; Yuehan Luo; Weikang Fu; Kai Yang

doi:10.1016/j.scitotenv.2024.171527

Interannual variations in ozone pollution with a dipole structure over Eastern China associated with springtime thermal forcing over the Tibetan Plateau

Sci Total Environ. 2024 May 1:923:171527. doi: 10.1016/j.scitotenv.2024.171527. Epub 2024 Mar 5.

Authors

Qingjian Yang¹, Tianliang Zhao², Yongqing Bai³, Jing Wei⁴, Xiaoyun Sun¹, Zhijie Tian⁵, Jun Hu⁶, Xiaodan Ma¹, Yuehan Luo¹, Weikang Fu¹, Kai Yang¹

Affiliations

¹ Climate and Weather Disasters Collaborative Innovation Center, Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, PREMIC, Nanjing University of Information Science &Technology, Nanjing 210044, China.
² Climate and Weather Disasters Collaborative Innovation Center, Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, PREMIC, Nanjing University of Information Science &Technology, Nanjing 210044, China. Electronic address: tlzhao@nuist.edu.cn.
³ Institute of Heavy Rain, China Meteorological Administration, Wuhan 430205, China.
⁴ Department of Atmospheric and Oceanic Science and ESSIC, University of Maryland, College Park, MD, USA.
⁵ China Institute for Radiation Protection, Taiyuan 030006, China.
⁶ Fujian Academy of Environmental Sciences, Fuzhou 350011, China.

PMID: 38453079
DOI: 10.1016/j.scitotenv.2024.171527

Abstract

The Tibetan Plateau (TP) is essential in modulating climate change in downstream Eastern China (EC). As a meteorology-sensitive pollutant, changes in ozone (O₃) in connection with the TP have received limited attention. In this study, using climate analysis of the China High Air Pollutants O₃ product and ERA5 reanalysis data of meteorology for 1980-2020, the effect of springtime TP thermal forcing on the warm season (April-September) O₃ pollution over EC was investigated. The strong TP thermal effect significantly modulates the interannual variations in O₃ pollution with a dipole pattern over EC, inducing more O₃ pollution in northern EC regions and alleviating O₃ pollution in the southern regions. In northern (southern) EC, strong TP thermal forcing triggers a significant anomalous high (low) pressure center accompanied by anticyclonic (cyclonic) anomalies, resulting in decreased (increased) total cloud cover, increased (reduced) surface downward solar radiation and air temperature, which are conducive to the anomalous increase (decrease) in surface O₃ concentrations. Moreover, the key sources of springtime thermal forcing over the TP influence the major O₃ pollution regions over southern and northern EC with an inverse pattern, depending on their locations and orientations to the large topography of the TP. This research reveals an important driving factor for the dipole interannual variation in O₃ pollution over EC, providing a new prospect for the effect of the TP on atmospheric environmental change.

Keywords: Climate variability; Ozone change; Spatial pattern; Thermal anomalies.