Flexible sensors have promising applications in the fields of health monitoring and artificial intelligence, which have attracted much attention from researchers. However, the design and manufacture of sensors with multiple sensing functions (like simultaneously having both temperature and pressure sensing capabilities) still present a significant challenge. Here, an ionic thermoelectric sensor for synchronous temperature and pressure sensing was developed on the basis of a carbon microtubes (CMTs)/potassium chloride (KCl)/gelatin composite consisting of gelatin as the polymer matrix, CMTs as the conductive material and KCl as the ion source. The designed CMTs/KCl/gelatin composite with the good ductility (830%) and flexibility can achieve a Seebeck coefficient of 4 mV K-1 and a dual stimulus responsiveness to pressure and temperature. In addition, not only the movement of the human body (e.g., fingers, arms), but also the temperature difference between the human body and the environment, were able to be monitored by the designed CMTs/KCl/gelatin sensors. This study provides a novel strategy for the design and preparation of high-performance flexible sensors by utilizing ion-gel thermoelectric materials and promotes the research of temperature and pressure sensing technologies.
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