2D Silver-Nanoplatelets Metasurface for Bright Directional Photoluminescence, Designed with the Local Kirchhoff's Law

ACS Nano. 2024 Feb 13;18(6):4903-4910. doi: 10.1021/acsnano.3c09874. Epub 2024 Jan 29.

Abstract

Semiconductor colloidal nanocrystals are excellent light emitters in terms of efficiency and spectral control. They can be integrated with a metasurface to make ultrathin photoluminescent devices with a reduced amount of active material and perform complex functionalities such as beam shaping or polarization control. To design such a metasurface, a quantitative model of the emitted power is needed. Here, we report the design, fabrication, and characterization of a ∼300 nm thick light-emitting device combining a plasmonic metasurface with an ensemble of nanoplatelets. The source has been designed with a methodology based on a local form of Kirchhoff's law. The source displays record high directionality and absorptivity.

Keywords: Kirchhoff; directionality; metasurfaces; nanoplatelets; photoluminescence.