Optical Bistability in Nanosilicon with Record Low Q-Factor

Nano Lett. 2023 Dec 27;23(24):11727-11733. doi: 10.1021/acs.nanolett.3c03597. Epub 2023 Nov 28.

Abstract

We demonstrated optical bistability in an amorphous silicon Mie resonator with a size of ∼100 nm and Q-factor as low as ∼4 by utilizing photothermal and thermo-optical effects. We not only experimentally confirmed the steep intensity transition and the hysteresis in the scattering response from silicon nanocuboids but also established a physical model to numerically explain the underlying mechanism based on temperature-dependent competition between photothermal heating and heat dissipation. The transition between the bistable states offered particularly steep superlinearity of scattering intensity, reaching an effective nonlinearity order of ∼100th power over excitation intensity, leading to the potential of advanced optical switching devices and super-resolution microscopy.

Keywords: Mie resonance; nanophotonics; optical nonlinearity; photothermal effect; silicon nanostructure.