Room-Temperature Zero-Field kπ- Skyrmions and Their Field-Driven Evolutions in Chiral Nanodisks

Nano Lett. 2023 Nov 22;23(22):10205-10212. doi: 10.1021/acs.nanolett.3c02746. Epub 2023 Nov 9.

Abstract

Target skyrmion, characterized by a central skyrmion surrounded by a series of concentric cylinder domains known as kπ-skyrmions (k ≥ 2), holds promise as a novel storage state in next-generation memories. However, target skyrmions comprising one or more concentric cylindrical domains have not been observed in chiral magnets, particularly at room temperature. In this study, we experimentally achieved kπ-skyrmions (k = 2, 3, and 4) with diameters of ∼220, 320, and 410 nm, respectively, and room-temperature stability under zero magnetic field by tightly confining these topological spin textures in β-Mn-type Co8Zn10Mn2 nanodisks. The magnetic configurations and their field-driven evolutions were simultaneously investigated by using in situ off-axis electron holography. In combination with numerical simulations, we further investigated the dependence of kmax on the nanodisk diameter. These findings highlight the potential of kπ-skyrmions as information carriers and offer insights into manipulation of kπ-skyrmions in the future.

Keywords: Co8Zn10Mn2; chiral magnet; kπ-skyrmions; off-axis electron holography.