Determining the Number of Graphene Nanoribbons in Dual-Gate Field-Effect Transistors

Nano Lett. 2023 Sep 27;23(18):8474-8480. doi: 10.1021/acs.nanolett.3c01931. Epub 2023 Sep 6.

Abstract

Bottom-up synthesized graphene nanoribbons (GNRs) are increasingly attracting interest due to their atomically controlled structure and customizable physical properties. In recent years, a range of GNR-based field-effect transistors (FETs) has been fabricated, with several demonstrating quantum-dot (QD) behavior at cryogenic temperatures. However, understanding the relationship between the cryogenic charge-transport characteristics and the number of the GNRs in the device is challenging, as the length and location of the GNRs in the junction are not precisely controlled. Here, we present a methodology based on a dual-gate FET that allows us to identify different scenarios, such as single GNRs, double or multiple GNRs in parallel, and a single GNR interacting with charge traps. Our dual-gate FET architecture therefore offers a quantitative approach for comprehending charge transport in atomically precise GNRs.

Keywords: charge-transport; field-effect transistors; graphene; nanoribbons.