Copper-Catalyzed Enantioselective and Regiodivergent Allylation of Ketones with Allenylsilanes

Angew Chem Int Ed Engl. 2023 Oct 26;62(44):e202311540. doi: 10.1002/anie.202311540. Epub 2023 Sep 18.

Abstract

We report herein a regiodivergent and enantioselective allyl addition to ketones with allenylsilanes through copper catalysis. With the combination of CuOAc, a Josiphos-type bidentate phosphine ligand and PhSiH3 , allyl addition to a variety of ketones furnishes branched products in excellent enantioselectivities. The regioselectivity is completely reversed by employing the P-stereogenic ligand BenzP*, affording the linear products with excellent enantioselectivities and good Z-selectivities. The linear Z-product could be converted to E-product via a catalytic geometric isomerization of the Z-alkene group. The silyl group in the products could provide a handle for downstream elaboration.

Keywords: Allenylsilanes; Allyl Addition; Enantioselective; Regiodivergent; Tertiary Homoallylic Alcohols.