Mobile monitoring is increasingly used to assess exposure to traffic-related air pollutants (TRAPs), including ultrafine particles (UFPs). Due to the rapid spatial decrease in the concentration of UFPs and other TRAPs with distance from roadways, mobile measurements may be non-representative of residential exposures, which are commonly used for epidemiologic studies. Our goal was to develop, apply, and test one possible approach for using mobile measurements in exposure assessment for epidemiology. We used an absolute principal component score model to adjust the contribution of on-road sources in mobile measurements to provide exposure predictions representative of cohort locations. We then compared UFP predictions at residential locations from mobile on-road plume-adjusted versus stationary measurements to understand the contribution of mobile measurements and characterize their differences. We found that predictions from mobile measurements are more representative of cohort locations after down-weighting the contribution of localized on-road plumes. Further, predictions at cohort locations derived from mobile measurements incorporate more spatial variation compared to those from short-term stationary data. Sensitivity analyses suggest that this additional spatial information captures features in the exposure surface not identified from the stationary data alone. We recommend the correction of mobile measurements to create exposure predictions representative of residential exposure for epidemiology.
Keywords: absolute principal component score; air pollution epidemiology; exposure assessment; prediction models; traffic-related air pollution; ultrafine particles.