Enabling Self-Induced Back-Action Trapping of Gold Nanoparticles in Metamaterial Plasmonic Tweezers

Nano Lett. 2023 Jun 14;23(11):4723-4731. doi: 10.1021/acs.nanolett.2c04492. Epub 2023 May 31.

Abstract

The pursuit for efficient nanoparticle trapping with low powers has led to optical tweezers technology moving from the conventional free-space configuration to advanced plasmonic systems. However, trapping nanoparticles smaller than 10 nm still remains a challenge even for plasmonic tweezers. Proper nanocavity design and excitation has given rise to the self-induced back-action (SIBA) effect offering enhanced trap stiffness with decreased laser power. In this work, we investigate the SIBA effect in metamaterial tweezers and its synergy with the exhibited Fano resonance. We demonstrate stable trapping of 20 nm gold particles with trap stiffnesses as high as 4.18 ± 0.2 (fN/nm)/(mW/μm2) and very low excitation intensity. Simulations reveal the existence of two different groups of hotspots on the plasmonic array. The two hotspots exhibit tunable trap stiffnesses, a unique feature that can allow for sorting of particles and biological molecules based on their characteristics.

Keywords: Fano resonance; gold nanoparticle trapping; metamaterial tweezers; plasmonic tweezers; self-induced back-action.