Strongly Coupled Magnon-Plasmon Polaritons in Graphene-Two-Dimensional Ferromagnet Heterostructures

Nano Lett. 2023 May 24;23(10):4510-4515. doi: 10.1021/acs.nanolett.3c00907. Epub 2023 May 11.

Abstract

Magnons and plasmons are different collective modes, involving the spin and charge degrees of freedom, respectively. Formation of hybrid plasmon-magnon polaritons in heterostructures of plasmonic and magnetic systems faces two challenges, the small interaction of the electromagnetic field of the plasmon with the spins, and the energy mismatch, as in most systems plasmons have energies orders of magnitude larger than those of magnons. We show that graphene plasmons form polaritons with the magnons of two-dimensional ferromagnetic insulators, placed up to to half a micrometer apart, with Rabi splittings in the range of 100 GHz (dramatically larger than cavity magnonics). This is facilitated both by the small energy of graphene plasmons and the cooperative super-radiant nature of the plasmon-magnon coupling afforded by phase matching. We show that the coupling can be modulated both electrically and mechanically, and we propose a ferromagnetic resonance experiment implemented with a two-dimensional ferromagnet driven by graphene plasmons.

Keywords: 2D magnets; FMR; magnons; plasmons; polaritons.