Fast One-Step Fabrication of Highly Regular Microscrolls with Controllable Surface Morphology

Adv Sci (Weinh). 2023 Jul;10(21):e2302103. doi: 10.1002/advs.202302103. Epub 2023 May 10.

Abstract

Although rolling origami technology has provided convenient access to three-dimensional (3D) microstructure systems, the high yield and scalable construction of complex rolling structures with well-defined geometry without impeding functionality has remained challenging. The straightforward, one-step fabrication that uses external mechanical stress to scroll micrometer thick, flexible planar films with centimeter lateral dimensions into tubular or spiral geometry within a few seconds is demonstrated. The method allows controlling the scrolls' diameter, number of windings and nanostructured surface morphology, and is applicable to a wide range of functional materials. The obtained 3D structures are highly promising for various applications including sensors, actuators, microrobotics, as well as energy storage and electronic devices.

Keywords: 3D microstructures; footprint; graphene oxide; microscrolls; nanocellulose; rolled-up nanotechnology; rolling; vanadium pentoxide.