A high concentration CO2 pool over the Indo-Pacific Warm Pool

Abstract

Anthropogenic emissions have produced significant amount of carbon dioxide (CO₂) in the atmosphere since the beginning of the industrial revolution. High levels of atmospheric CO₂ increases global temperature as CO₂ absorbs outgoing longwave radiation and re-emits. Though a well-mixed greenhouse gas, CO₂ concentration is not uniform in the atmosphere across different altitudes and latitudes. Here, we uncover a region of high CO₂ concentration (i.e. CO₂ pool) in the middle troposphere (500-300 hPa) over the Indo-Pacific Warm Pool (IPWP, 40° E-140° W, 25° S-25° N), in which the CO₂ concentration is higher than that of other regions in the same latitude band (20° N-20° S), by using CO₂ satellite measurements for the period 2002-2017. This CO₂ pool extends from the western Pacific to the eastern Indian Ocean. Much of the CO₂ pool is over the western Pacific Ocean (74.87%), and the remaining lies over the eastern Indian Ocean (25.13%). The rising branch of Walker circulation acts as a "CO₂ Chimney" that constantly transports CO₂ released from the natural, human-induced and ocean outgassing processes to the middle and upper troposphere. The CO₂ pool evolves throughout the year with an average annual trend of about 2.17 ppm yr^-1, as estimated for the period 2003-2016. Our analysis further reveals that La Niña (El Niño) events strengthen (weaken) the CO₂ pool in the mid-troposphere. The radiative forcing for the CO₂ pool suggests more warming in the region and is a grave concern for global warming and climate change.