High-Entropy Perovskites for Energy Conversion and Storage: Design, Synthesis, and Potential Applications

Yuhao Wang; Jiapeng Liu; Yufei Song; Jing Yu; Yunfeng Tian; Matthew James Robson; Jian Wang; Zhiqi Zhang; Xidong Lin; Guodong Zhou; Zheng Wang; Longyun Shen; Hailei Zhao; Salvatore Grasso; Francesco Ciucci

doi:10.1002/smtd.202201138

High-Entropy Perovskites for Energy Conversion and Storage: Design, Synthesis, and Potential Applications

Small Methods. 2023 Apr;7(4):e2201138. doi: 10.1002/smtd.202201138. Epub 2023 Feb 26.

Authors

Yuhao Wang¹, Jiapeng Liu¹, Yufei Song¹, Jing Yu¹, Yunfeng Tian¹, Matthew James Robson¹, Jian Wang², Zhiqi Zhang¹, Xidong Lin^{1

3}, Guodong Zhou¹, Zheng Wang¹, Longyun Shen^{1

4}, Hailei Zhao^{5

6}, Salvatore Grasso⁷, Francesco Ciucci^{1

8

9}

Affiliations

¹ Department of Mechanical and Aerospace Engineering, The Hong Kong University of Science and Technology, Hong Kong SAR, P. R. China.
² School of Energy and Environment, City University of Hong Kong, Kowloon, Hong Kong SAR, P. R. China.
³ Julong College, Shenzhen Technology University, Shenzhen, 518118, P. R. China.
⁴ Division of Emerging Interdisciplinary Areas, Hong Kong University of Science and Technology, Hong Kong SAR, P. R. China.
⁵ School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing, 100083, P. R. China.
⁶ Beijing Municipal Key Lab for Advanced Energy Materials and Technologies, Beijing, 100083, P. R. China.
⁷ Key Laboratory of Advanced Technologies of Materials, Ministry of Education, School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu, 610031, P. R. China.
⁸ HKUST Shenzhen-Hong Kong Collaborative Innovation Research Institute, Shenzhen, 518048, P. R. China.
⁹ Energy Institute, The Hong Kong University of Science and Technology, Hong Kong SAR, P. R. China.

PMID: 36843320
DOI: 10.1002/smtd.202201138

Abstract

Perovskites have shown tremendous promise as functional materials for several energy conversion and storage technologies, including rechargeable batteries, (electro)catalysts, fuel cells, and solar cells. Due to their excellent operational stability and performance, high-entropy perovskites (HEPs) have emerged as a new type of perovskite framework. Herein, this work reviews the recent progress in the development of HEPs, including synthesis methods and applications. Effective strategies for the design of HEPs through atomistic computations are also surveyed. Finally, an outlook of this field provides guidance for the development of new and improved HEPs.

Keywords: applications; computational understanding; energy conversion; energy storage; high-entropy perovskites; synthetic methods.

Publication types

Review

Abstract

Publication types

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