Nanocellulose/polyethylenimine composites have attracted growing attention due to their versatility as new materials for application in different fields. Water remediation is one of the traditional applications of these composites and their investigation as adsorbents for single water pollutants is well established. However, most water resources such as rivers, lakes, and even oceans contain complex mixtures of pollutants. Despite several recently published reviews on water purification technology, they only focused on these material as single pollutant removers and hardly mentioned their capacity to simultaneously recover multiple pollutants. Therefore, there is still a gap in the archived literature considering nanocellulose/polyethylenimine composites targeting water remediation with multiple water pollutants. In this review, methods for synthesizing such composites are classified and compared according to the mechanism of reactions, such as chemical crosslinking and physical adsorption, while outlining advantages and limitations. Then, the water pollutants mainly targeted by those composites are discussed in detail to expound the relationship between the synthesis method and the type and adsorption capacity. Finally, the last section presents challenges and opportunities of these nanocellulose/polyethylenimine composites as emerging sorbents for sustainable multiple water pollutants purification technologies. This review aims to lay out the basis for future developments of these composites for multiple water pollutants.
Keywords: Adsorption; Bio-based adsorbents; Covalent bonding; Crosslinking; Water remediation.
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