Long-term core-mantle interaction explains W-He isotope heterogeneities

Proc Natl Acad Sci U S A. 2023 Jan 24;120(4):e2215903120. doi: 10.1073/pnas.2215903120. Epub 2023 Jan 17.

Abstract

The isotopic characteristics of ocean island basalts have long been used to infer the nature of their source and the long-term evolution of the Earth's mantle. Anticorrelation between tungsten and helium isotopic signatures is a particularly puzzling feature in those basalts, which no single process appears to explain. Traditionally, the high 3He/4He signature has been attributed to an undegassed reservoir in the deep mantle. Additional processes needed to obtain low 182W/184W often entail unobserved ancillary geochemical effects. It has been suggested, however, that the core feeds the lower mantle with primordial helium, obviating the need for an undegassed mantle reservoir. Independently, the tungsten-rich core has been suggested to impart the plume source with anomalous tungsten isotope signatures. We advance the idea that isotopic diffusion may simultaneously transport both tungsten and helium across the core-mantle boundary, with the striking implication that diffusion can naturally account for the observed isotopic trend. By modeling the long-term isotopic evolution of mantle domains, we demonstrate that this mechanism can account for more than sufficient isotopic ratios in plume-source material, which, after dynamical transport to the Earth's surface, are consistent with the present-day mantle W-He isotopic heterogeneities. No undegassed mantle reservoir is required, bearing significance on early Earth conditions such as the extent of magma oceans.

Keywords: core; entrainment; helium; isotope heterogeneity; tungsten.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Diffusion
  • Helium*
  • Isotopes
  • Tungsten*

Substances

  • Helium
  • Tungsten
  • basalt
  • Isotopes