Migration behaviour of LNAPL in fractures filled with porous media: Laboratory experiments and numerical simulations

Huan Shen; Yong Huang; Walter A Illman; Yue Su; Kehan Miao

doi:10.1016/j.jconhyd.2022.104118

Migration behaviour of LNAPL in fractures filled with porous media: Laboratory experiments and numerical simulations

J Contam Hydrol. 2023 Feb:253:104118. doi: 10.1016/j.jconhyd.2022.104118. Epub 2022 Nov 25.

Authors

Huan Shen¹, Yong Huang², Walter A Illman³, Yue Su⁴, Kehan Miao⁵

Affiliations

¹ School of Earth Sciences and Engineering, Hohai University, Nanjing 210098, China; Department of Earth and Environmental Sciences, University of Waterloo, Waterloo N2L 3G1, Canada. Electronic address: shenh@hhu.edu.cn.
² School of Earth Sciences and Engineering, Hohai University, Nanjing 210098, China. Electronic address: hyong@hhu.edu.cn.
³ Department of Earth and Environmental Sciences, University of Waterloo, Waterloo N2L 3G1, Canada. Electronic address: willman@uwaterloo.ca.
⁴ School of Earth Sciences and Engineering, Hohai University, Nanjing 210098, China; Department of Earth and Environmental Sciences, University of Waterloo, Waterloo N2L 3G1, Canada. Electronic address: suyue@hhu.edu.cn.
⁵ School of Earth Sciences and Engineering, Hohai University, Nanjing 210098, China. Electronic address: miaokh2021@hhu.edu.cn.

PMID: 36563651
DOI: 10.1016/j.jconhyd.2022.104118

Abstract

With the increasing requirement of maintaining world energy security and strategic reserves, oil storage and transportation facilities are being built at a large scale. Taking the safe and efficient operation of petroleum storage projects as the goal, a set of experimental apparatus to investigate the migration of contaminants in fractures filled with media was developed to predict and evaluate the environmental risk of oil contaminants leakage. A multiphase numerical flow model based on COMSOL was built based on the laboratory experimental model. Specifically, the migration behaviour of Light Non-aqueous Phase Liquid (LNAPL) through a sand-filled fractured medium was studied by laboratory experiments and numerical simulations. Image and chemical analyses methods were used to monitor and study LNAPL migration behaviour for varying grain sizes of porous medium filling the fractures and varying groundwater table elevations. Laboratory experimental results showed that the LNAPL migration velocity in filled fracture network was significantly faster than that in adjoining porous media during the initial stage of infiltration. The migration velocity increased with the relative permeability of filled sand, which was closely related to the Van Genuchten (VG) model parameters α and n. LNAPL migrated downward with the falling groundwater table and became entrapped with the rising groundwater table, and the amount of entrapment depended on VG model parameters. Hydrogeological parameters were calibrated and LNAPL migration in filled fractured media was predicted using the calibrated numerical model. Simulation results revealed that fracture inclination had an important influence on LNAPL migration in filled fractured media and its migration velocity decreased with a decrease in fracture inclination. These research results can be applied to the control and remediation of oil-contaminated sites in fractured rock settings, such as at underground oil storage tanks and caverns, as well as at underground oil pipelines.

Keywords: Contaminant migration; Fractures filled with porous media; Laboratory experiment; Light non-aqueous phase liquid (LNAPL); Numerical simulation.

Publication types

Research Support, Non-U.S. Gov't

MeSH terms

Computer Simulation
Groundwater*
Models, Theoretical
Porosity
Sand*

Substances

Sand