Typhoon triggers estuarine heavy metal risk by regulating the multifractal grainsize of resuspended sediment

Sci Total Environ. 2023 Feb 20:860:160510. doi: 10.1016/j.scitotenv.2022.160510. Epub 2022 Nov 28.

Abstract

The turbulent boundary layer generated by wind in the estuarine surface water serves as a main factor affecting the distribution of suspended particulate matter (SPM) and suspended sediment concentration (SSC). In this study, representative typhoon-induced variation of surface fine SPM (<63 μm) was simulated in the Yangtze River Estuary (YRE) under two time scenarios. Each scenario contained four grainsize SPM fractions named Fraction 1 (<8 μm), Fraction 2 (8-16 μm), Fraction 3 (16-32 μm), Fraction 4 (32-63 μm). The typhoon-induced resuspended multifractal SSC quantification (TRMSQ) based on the relationship between SPM grainsize and heavy metal adsorption capacity was proposed to assess the variation in the resuspended threat of heavy metal to 6 key estuarine protected objects (three reservoirs & three national reserves) between Scenarios 1 and 2. The results presented that Fraction 3 exhibited the maximum increment in SSC resuspension mass and longest regression time from typhoon. Combined with TRMSQ, chromium (Cr) was calculated to be the riskiest typhoon-induced factor. The integrated resuspended risk of heavy metals for each protected object tends to increase from the northwest of Chongming Island (1.2) towards the maximum turbidity zone (>9) downstream, with an estuary-wide mean of 3.3.

Keywords: Estuary; Grainsize grading simulation; Heavy metal risk; Sediment resuspension; Typhoon.

MeSH terms

  • China
  • Cyclonic Storms*
  • Environmental Monitoring / methods
  • Estuaries
  • Geologic Sediments
  • Metals, Heavy* / analysis
  • Particulate Matter / analysis
  • Water Pollutants, Chemical* / analysis

Substances

  • Water Pollutants, Chemical
  • Metals, Heavy
  • Particulate Matter