α-Acylation of Alkenes by a Single Photocatalyst

Angew Chem Int Ed Engl. 2022 Dec 23;61(52):e202208831. doi: 10.1002/anie.202208831. Epub 2022 Nov 24.

Abstract

A direct strategy for the difunctionalization of alkenes, with acylation occurring at the more substituted alkene position, would be attractive for complex ketone synthesis. We report herein a reaction driven by a single photocatalyst that enables α-acylation in this way with the introduction of a fluoromethyl, alkyl, sulfonyl or thioether group at the β-position of the alkene with high chemo- and regioselectivity under extremely mild conditions. Crucial to the success of this method are rate differences in the kinetics of radical generation through single-electron transfer (SET) between different radical precursors and the excited photocatalyst (PC*). Thus, the β-position of the alkene is first occupied by the group derived from the radical precursor that can be generated most readily, and α-keto acids could be used as an electrophilic reagent for the α-acylation of alkenes.

Keywords: Alkenes; Difunctionalization; Photocatalysis; Reaction Kinetics; Synthetic Methods.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acylation
  • Alkenes*
  • Catalysis
  • Indicators and Reagents

Substances

  • Alkenes
  • Indicators and Reagents