Plasmon-Enhanced Fluorescence Emission of an Electric Dipole Modulated by a Nanoscale Silver Hemisphere

Nanomaterials (Basel). 2022 Sep 3;12(17):3070. doi: 10.3390/nano12173070.

Abstract

The spontaneous emission of a fluorophore is altered by the surrounding electromagnetic field. Therefore, the radiation of the fluorophore can be engineered by inter-coupling with the nanoscale plasmons. This work proposes a nanoscale hemisphere structure that enhances the electric field and further modulates its effects on fluorophores by adjusting the radius of the hemisphere. A full-wave simulation is carried out using the finite element method, and the radiation characteristics of the nanoscale hemisphere are studied in detail. Compared with free space, the structure has generated significant enhancement exceeding 30. Through curve fitting, the relationship between the enhanced peak wavelength and the radius of the hemisphere is obtained.

Keywords: fluorescence enhancement; nanoscale hemisphere; surface plasmon.