Spin-Labeled Riboswitch Synthesized from a Protected TPA Phosphoramidite Building Block

Chemistry. 2022 Oct 7;28(56):e202201822. doi: 10.1002/chem.202201822. Epub 2022 Aug 18.

Abstract

The nitroxide TPA (2,2,5,5-tetramethyl-pyrrolin-1-oxyl-3-acetylene) is an excellent spin label for EPR studies of RNA. Previous synthetic methods, however, are complicated and require special equipment. Herein, we describe a uridine derived phosphoramidite with a photocaged TPA unit attached. The light sensitive 2-nitrobenzyloxymethyl group can be removed in high yield by short irradiation at 365 nm. Based on this approach, a doubly spin-labeled 27mer neomycin sensing riboswitch was synthesized and studied by PELDOR. The overall thermal stability of the fold is not much reduced by TPA. In-line probing nevertheless detected changes in local mobility.

Keywords: PELDOR; RNA aptamer; nitroxide; photocaged spin label; secondary structure mapping.

MeSH terms

  • Alkynes
  • Electron Spin Resonance Spectroscopy / methods
  • Neomycin
  • Organophosphorus Compounds
  • RNA
  • Riboswitch*
  • Spin Labels
  • Uridine

Substances

  • Alkynes
  • Organophosphorus Compounds
  • Riboswitch
  • Spin Labels
  • phosphoramidite
  • RNA
  • Neomycin
  • Uridine