Atmospheric pollution refers to the presence of substances in the air such as particulate matter (PM) which has a negative impact in population ́s health exposed to it. This makes it a topic of current interest. Since the Metropolitan Zone of the Valley of Mexico's geographic characteristics do not allow proper ventilation and due to its population's density a significant quantity of poor air quality events are registered. This paper proposes a methodology to improve the forecasting of PM10 and PM2.5, in largely populated areas, using a recurrent long-term/short-term memory (LSTM) network optimized by the Ant Colony Optimization (ACO) algorithm. The experimental results show an improved performance in reducing the error by around 13.00% in RMSE and 14.82% in MAE using as reference the averaged results obtained by the LSTM deep neural network. Overall, the current study proposes a methodology to be studied in the future to improve different forecasting techniques in real-life applications where there is no need to respond in real time.Implications: This contribution presents a methodology to deal with the highly non-linear modeling of airborne particulate matter (both PM10 and PM2.5). Most linear approaches to this modeling problem are often not accurate enough when dealing with this type of data. In addition, most machine learning methods require extensive training or have problems when dealing with noise embedded in the time-series data. The proposed methodology deals with this data in three stages: preprocessing, modeling, and optimization. In the preprocessing stage, data is acquired and imputed any missing data. This ensures that the modeling process is robust even when there are errors in the acquired data and is invalid, or the data is missing. In the modeling stage, a recurrent deep neural network called LSTM (Long-Short Term Memory) is used, which shows that regardless of the monitoring station and the geographical characteristics of the site, the resulting model shows accurate and robust results. Furthermore, the optimization stage deals with enhancing the capability of the data modeling by using swarm intelligence algorithms (Ant Colony Optimization, in this case). The results presented in this study were compared with other works that presented traditional algorithms, such as multi-layer perceptron, traditional deep neural networks, and common spatiotemporal models, which show the feasibility of the methodology presented in this contribution. Lastly, the advantages of using this methodology are highlighted.