The formation of self-cleaning functions on silicone elastomers is crucial for practical applications but still challenging. In this study, superhydrophobic silicone elastomers (SHSEs) with a 3D-hierarchical microstructure were achieved during the curing process with the assistance of a homemade template. The micro-nano structure formed by the assistance of the template makes the silicone elastomer surface achieve robust superhydrophobicity with a WCA at ∼163°, which can easily self-clean, removing surface contamination. Also, TiO2 particles transferred from the template endow the surface with photocatalytic functions, which can degrade organic pollutants under UV irradiation. After sandpaper abrasion, the formed SHSE can maintain its excellent hydrophobicity and show liquid repellency to wine and coffee droplets. The SHSEs with self-cleaning functions have promising applications in water treatment, medical facilities, and wearable devices.
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