To improve the energy efficiency and driving performance of ionic electroactive polymer actuators, we propose inserting insulating layers of 170 nm hexagonal boron nitride (h-BN) particles between the ionic polymer membrane and electrodes. In experiments, actuators exhibited better capacitance (4.020 × 10-1 F), displacement (6.01 mm), and curvature (35.59 m-1) with such layers than without them. The excellent insulating properties and uniform morphology of the layers reduced the interfacial resistance, and the ion conductivity (0.071 S m-1) within the ionic polymer improved significantly. Durability was enhanced because the h-BN layer is chemically and thermally stable and efficiently blocks heat diffusion and ion hydrate evaporation during operation. The results demonstrate a close relationship between the capacitance and driving performance of actuators. A gripper prepared from the proposed ionic electroactive polymer actuator can stably hold an object even under strong external vibration and fast or slow movement.
Keywords: acuators; artificial muscle; capacitance; electrochemistry; insulators; interface structure; ionic electroactivepolymers; mechanical properties.