Relaxation Oscillations of an Exciton-Polariton Condensate Driven by Parametric Scattering

Nano Lett. 2022 Apr 13;22(7):3026-3032. doi: 10.1021/acs.nanolett.2c00235. Epub 2022 Mar 28.

Abstract

We report the observation of coherent oscillations in the relaxation dynamics of an exciton-polariton condensate that were driven by parametric scattering processes. As a result of the interbranch scattering scheme and the nonlinear polariton-polariton interactions, such parametric scatterings exhibit a high scattering efficiency that leads to the fast depletion of the polariton condensate and the periodic shut-off of the bosonic stimulation processes, eventually causing relaxation oscillations. Employing polariton-reservoir interactions, the oscillation dynamics in the time domain can be projected onto the energy space. In theory, our simulations using the open-dissipative Gross-Pitaevskii equation are in excellent agreement with experimental observations. Surprisingly, the oscillation patterns, including many excitation pulses, are clearly visible in our time-integrated images, implying the high stability of the relaxation oscillations driven by polariton parametric scatterings.

Keywords: Gross−Pitaevskii equation; condensate; exciton−polariton; parametric scattering; relaxation oscillation.