Phase-locking of time-delayed attosecond XUV pulse pairs

Opt Express. 2022 Feb 28;30(5):7082-7095. doi: 10.1364/OE.452018.

Abstract

We present a setup for the generation of phase-locked attosecond extreme ultraviolet (XUV) pulse pairs. The attosecond pulse pairs are generated by high harmonic generation (HHG) driven by two phase-locked near-infrared (NIR) pulses that are produced using an actively stabilized Mach-Zehnder interferometer compatible with near-single cycle pulses. The attosecond XUV pulses can be delayed over a range of 400 fs with a sub-10-as delay jitter. We validate the precision and the accuracy of the setup by XUV optical interferometry and by retrieving the energies of Rydberg states of helium in an XUV pump-NIR probe photoelectron spectroscopy experiment.