Elliptic dichroism in strong-field ionization of atoms subjected to tailored laser fields

Phys Chem Chem Phys. 2022 Mar 16;24(11):7014-7027. doi: 10.1039/d1cp05209h.

Abstract

The differential ionization rate for strong-field ionization by tailored laser fields of atomic systems averaged over the magnetic quantum number satisfies particular inversion and reflection symmetries. The symmetries of the elliptic-dichroism parameter, which is related to the change of sign of the ellipticity of the laser field, are considered in detail, with particular emphasis on high-order above-threshold ionization. The general results are illustrated by the examples of an elliptically polarized laser field and a bi-elliptical orthogonally polarized two-color (BEOTC) field. For the BEOTC field the differential ionization rate and the elliptic-dichroism parameter are investigated for the ω-2ω and ω-3ω field combinations and for various relative phases between the laser-field components. The inversion and reflection symmetries of the photoelectron momentum distribution in the polarization plane of the field depend on the parities of r and s in the -- BEOTC field combination and on the relative phase between the field components. We suggest that, by analyzing the symmetry properties of the measured momentum distribution of the elliptic-dichroism parameter, one can identify the mechanism of strong-field ionization. If the rescattering mechanism is dominant one can use these distributions to obtain information about the atomic and molecular structure and dynamics.