Visible light communication (VLC), combining wireless communication with white lighting, has many advantages. It is free of electromagnetic interference, is rich in spectrum resources, and has a gigabit-per-second (Gbps) data rate. Laser diodes (LDs) are emerging as promising light sources for high-speed VLC communication due to their high modulation bandwidth. In this paper, we demonstrate a red/green/blue (R/G/B) LDs based VLC system with a recorded data rate of 46.41 Gbps, employing discrete multitone (DMT) and adaptive bit-loading technology to achieve high spectral efficiency (SE). The emission characteristics and transmission performance of R/G/B-LDs are discussed. The optimal data rates of R/G/B-LDs channels are 17.168/14.652/14.590 Gbps, respectively. The bit-error-ratio (BER) of each channel satisfies the 7% forward-error-correction (FEC) threshold (3.8×10-3) and greatly approaches the channel Shannon limit.