Accurate real-time monitoring of fine dust using a densely connected convolutional networks with measured plasma emissions

Chemosphere. 2022 Apr:293:133604. doi: 10.1016/j.chemosphere.2022.133604. Epub 2022 Jan 13.

Abstract

Accurate identification and monitoring of fine dust are emerging as a primary global issue for addressing the harmful effects of fine dust on public health. Identifying the source of fine dust is indispensable for ensuring the human lifespan as well as preventing environmental disasters. Here a simple yet effective spark-induced plasma spectroscopy (SIPS) unit combined with deep learning for real-time classification is verified as a fast and precise PM (particulate matter) source identification technique. SIPS promises portable use, label-free detection, source identification, and chemical susceptibility in a single step with acceptable speed and accuracy. In particular, the densely connected convolutional networks (DenseNet) are used with measured spark-induced plasma emission datasets to identify PM sources at above 98%. The identification performance was compared with other common classification methods, and DenseNet with dropouts (30%), optimized batch size (16), and cyclic learning rate training emerged as the most promising source identification method.

Keywords: Deep learning; DenseNet; Fine dust; Source identification; Spark-induced plasma spectroscopy.

MeSH terms

  • Air Pollutants* / analysis
  • Dust* / analysis
  • Environmental Monitoring / methods
  • Humans
  • Particulate Matter / analysis
  • Spectrum Analysis
  • Vehicle Emissions / analysis

Substances

  • Air Pollutants
  • Dust
  • Particulate Matter
  • Vehicle Emissions