Forecasting ambient PM2.5 concentrations with spatiotemporal coverage is key to alerting decision makers of pollution episodes and preventing detrimental public exposure, especially in regions with limited ground air monitoring stations. The existing methods rely on either chemical transport models (CTMs) to forecast spatial distribution of PM2.5 with nontrivial uncertainty or statistical algorithms to forecast PM2.5 concentration time series at air monitoring locations without continuous spatial coverage. In this study, we developed a PM2.5 forecast framework by combining the robust Random Forest algorithm with a publicly accessible global CTM forecast product, NASA's Goddard Earth Observing System "Composition Forecasting" (GEOS-CF), providing spatiotemporally continuous PM2.5 concentration forecasts for the next 5 days at a 1 km spatial resolution. Our forecast experiment was conducted for a region in Central China including the populous and polluted Fenwei Plain. The forecast for the next 2 days had an overall validation R2 of 0.76 and 0.64, respectively; the R2 was around 0.5 for the following 3 forecast days. Spatial cross-validation showed similar validation metrics. Our forecast model, with a validation normalized mean bias close to 0, substantially reduced the large biases in GEOS-CF. The proposed framework requires minimal computational resources compared to running CTMs at urban scales, enabling near-real-time PM2.5 forecast in resource-restricted environments.
Keywords: Random Forest; XGBoost; air pollution forecast; chemical transport model; near-real-time; near-term.