Reparametrization of the Colle-Salvetti formula

R Soc Open Sci. 2022 Jan 5;9(1):211333. doi: 10.1098/rsos.211333. eCollection 2022 Jan.

Abstract

We investigate the Colle-Salvetti (CS) formula, the basis of the Lee, Yang and Parr (LYP) correlation functional used in approximate density functional theory. The CS formula is reparametrized using high-accuracy Hartree-Fock (HF) wavefunctions to determine the accuracy of the formula to calculate anions. Fitting to the hydride ion or the two-electron system just prior to electron detachment at the HF level of theory does not, in general, improve the calculated correlation energies using the parameters derived from the CS/LYP method. An analysis of the CS parameters used in the popular LYP functional demonstrates the ingenuity and perhaps fortuitousness of the original formulation by CS.

Keywords: Hartree–Fock critical nuclear charge; Hartree–Fock wavefunctions; anion correlation energy; correlation energy formulae; electron correlation.

Associated data

  • figshare/10.6084/m9.figshare.c.5754025