From Low-Field Sondheimer Oscillations to High-Field Very Large and Linear Magnetoresistance in a SrTiO3-Based Two-Dimensional Electron Gas

Nano Lett. 2022 Jan 12;22(1):65-72. doi: 10.1021/acs.nanolett.1c03198. Epub 2021 Dec 16.

Abstract

Quantum materials harbor a cornucopia of exotic transport phenomena challenging our understanding of condensed matter. Among these, a giant, nonsaturating linear magnetoresistance (MR) has been reported in various systems, from Weyl semimetals to topological insulators. Its origin is often ascribed to unusual band structure effects, but it may also be caused by extrinsic sample disorder. Here, we report a very large linear MR in a SrTiO3 two-dimensional electron gas and, by combining transport measurements with electron spectromicroscopy, show that it is caused by nanoscale inhomogeneities that are self-organized during sample growth. Our data also reveal semiclassical Sondheimer oscillations arising from interferences between helicoidal electron trajectories, from which we determine the 2DEG thickness. Our results bring insight into the origin of linear MR in quantum materials, expand the range of functionalities of oxide 2DEGs, and suggest exciting routes to explore the interaction of linear MR with features like Rashba spin-orbit coupling.

Keywords: 2D electron gas; Sondheimer oscillations; linear magnetoresistance; oxide interfaces.