Aerosol optical properties and its type classification based on multiyear joint observation campaign in north China plain megalopolis

Yu Zheng; Huizheng Che; Xiangao Xia; Yaqiang Wang; Leiku Yang; Jing Chen; Hong Wang; Hujia Zhao; Lei Li; Lei Zhang; Ke Gui; Xianyi Yang; Yuanxin Liang; Xiaoye Zhang

doi:10.1016/j.chemosphere.2020.128560

Aerosol optical properties and its type classification based on multiyear joint observation campaign in north China plain megalopolis

Chemosphere. 2020 Oct 8:128560. doi: 10.1016/j.chemosphere.2020.128560. Online ahead of print.

Authors

Yu Zheng¹, Huizheng Che², Xiangao Xia³, Yaqiang Wang¹, Leiku Yang⁴, Jing Chen⁵, Hong Wang¹, Hujia Zhao⁶, Lei Li¹, Lei Zhang¹, Ke Gui¹, Xianyi Yang¹, Yuanxin Liang¹, Xiaoye Zhang¹

Affiliations

¹ State Key Laboratory of Severe Weather (LASW) and Key Laboratory of Atmospheric Chemistry (LAC), Chinese Academy of Meteorological Sciences, CMA, Beijing, 100081, China.
² State Key Laboratory of Severe Weather (LASW) and Key Laboratory of Atmospheric Chemistry (LAC), Chinese Academy of Meteorological Sciences, CMA, Beijing, 100081, China. Electronic address: chehz@cma.gov.cn.
³ Laboratory for Middle Atmosphere and Global Environment Observation (LAGEO), Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing, 100029, China; School of Geoscience, University of Chinese Academy of Science, Beijing, 100049, China.
⁴ School of Surveying and Land Information Engineering, Henan Polytechnic University, Jiaozuo, 454000, China.
⁵ Shijiazhuang Meteorological Bureau, Shijiazhuang, 050081, China.
⁶ Institute of Atmospheric Environment, China Meteorological Administration, Shenyang, 110016, China.

PMID: 34756345
DOI: 10.1016/j.chemosphere.2020.128560

Abstract

Since haze and other air pollution are frequently seen in the North China Plain (NCP), detail information on aerosol optical and radiative properties and its type classification is demanded for the study of regional environmental pollution. Here, a multiyear ground-based synchronous sun photometer observation at seven sites on North China Plain megalopolis from 2013 to 2018 was conducted. First, the annual and seasonal variation of these characteristics as well as the intercomparsion were analyzed. Then the potential relationships between these properties with meteorological factors and the aerosol type classification were discussed. The results show: Particle volume exhibited a decreasing trend from the urban downtown to suburban and the rural region. The annual average aerosol optical depth at 440 nm (AOD₄₄₀) varied from ∼0.43 to 0.86 over the NCP. Annual average single-scattering albedo at 440 nm (SSA₄₄₀) varied from ∼0.89 to 0.93, indicating a moderate to slight absorption capacity. Average absorption aerosol optical depth at 440 nm (AAOD₄₄₀) varied from ∼0.07 to 0.10. The absorption Ångström exponent (AAE) (∼0.89-1.40) indicated the multi-types of absorptive matters originated form nature and anthropogenic emission. The discussion of aerosol composition showed a smaller particle size of aerosol from biomass burning and/or fossil foil consumption with enhanced aerosol scattering and enlarged light extinction. Aerosol classification indicated a large percentage of mixed absorbing aerosol (∼20%-49%), which showed increasing trend between relative humidity (RH) with aerosol scattering and dust was an important environmental pollutant compared to southern China.

Keywords: Aerosol optical properties; Ground-based observation; Megalopolis; North China Plain; Type classification.