Visualization of Subatomic Movements in Nanostructures

Nano Lett. 2021 Sep 22;21(18):7746-7752. doi: 10.1021/acs.nanolett.1c02644. Epub 2021 Sep 1.

Abstract

Electron microscopy, scanning probe, and optical super-resolution imaging techniques with nanometric resolution are now routinely available but cannot capture the characteristically fast (MHz-GHz frequency) movements of micro-/nano-objects. Meanwhile, optical interferometric techniques can detect high-frequency picometric displacements but only with diffraction-limited lateral resolution. Here, we introduce a motion visualization technique, based on the spectrally resolved detection of secondary electron emission from moving objects, that combines picometric displacement sensitivity with the nanometric spatial (positional/imaging) resolution of electron microscopy. The sensitivity of the technique is quantitatively validated against the thermodynamically defined amplitude of a nanocantilever's Brownian motion. It is further demonstrated in visualizing externally driven modes of cantilever, nanomechanical photonic metamaterial, and MEMS device structures. With a noise floor reaching ∼1 pm/Hz1/2, it can provide for the study of oscillatory movements with subatomic amplitudes, presenting new opportunities for the interrogation of motion in functional structures across the materials, bio- and nanosciences.

Keywords: electron microscopy; metrology; nanomechanics; thermal motion.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Microscopy, Electron
  • Motion
  • Nanostructures*
  • Optical Imaging
  • Photons