Assessment of residual radionuclide levels at the Bokak and Bikar Atolls in the northern Marshall Islands

Abstract

The Bikar and Bokak Atolls, located in the northern Marshall Islands, are extremely isolated and consist of pristine marine and terrestrial ecosystems. Both atolls may have experienced significant radioactive deposition following the nuclear weapon testing conducted at Bikini and Enewetak proving grounds. Here we report activity concentrations of artificial radionuclides (²³⁹Pu, ²⁴⁰Pu, ²⁴¹Pu, ²⁴¹Am, ¹³⁷Cs and ⁹⁰Sr) in marine and terrestrial samples collected from Bikar and Bokak Atolls. Artificial radionuclides in soil from the Majuro Atoll are also reported and form a radiological baseline against which the levels at the other atolls can be compared. We observed low levels of artificial radionuclides in soil from Majuro and Bokak, but significantly higher levels in soil from Bikar. The residual radioactivity in the Bikar environment is comparable to the levels previously reported for other nearby atolls, including Taka and Utrik, but lower than for Rongerik, Rongelap, Bikini and Enewetak. An analysis of ²⁴⁰Pu/²³⁹Pu isotope ratios and estimations of the dates of contamination from ²⁴¹Am/²⁴¹Pu activity ratios both indicated that the Bikar Atoll was contaminated mainly by radioactive fallout from the Castle Bravo test in 1954. We compare the results of our measurements at Bikar and Bokak to data from other atolls in the Marshall Islands and to regions of the world affected by both global and regional fallout from atmospheric nuclear weapons testing and nuclear accidents.

Keywords: (240)Pu/(239)Pu ratio; (241)Am/(241)Pu age; Marshall Islands; Nuclear weapon tests; Pristine ecosystems; Residual radioactivity.