A record of fallout 239Pu and 240Pu at World Heritage Bathurst Harbour, Tasmania, Australia

Abstract

This study presents the first measurements of anthropogenic plutonium (²³⁹Pu and ²⁴⁰Pu) concentrations and atom ratios (²⁴⁰Pu/²³⁹Pu) for Tasmania, in sediment collected from Bathurst Harbour, in the Tasmanian Wilderness World Heritage Area, Australia. The weighted mean ²⁴⁰Pu/²³⁹Pu atom ratio measured at this site was 0.172 ± 0.007 which is consistent with published data from mainland Australia and global and Southern Hemisphere averages. The ²⁴⁰Pu/²³⁹Pu atom ratios ranged between 0.11 and 0.21 with the earliest recorded ²⁴⁰Pu/²³⁹Pu atom ratios being the lowest, suggesting an influence of low atom ratio fallout from nuclear testing in Australia. Post-moratorium fallout ²⁴⁰Pu/²³⁹Pu atom ratios were consistent with other records. Lead-210 (²¹⁰Pb) sediment chronologies indicate sediment accumulation rates have increased since the early part of the 19th century at this location.

Keywords: (210)Pb; (239)Pu; (240)Pu; AMS; Fallout radionuclide; Plutonium; Sedimentation.