Functional resins with optical adjustment capability own great potential in multiple application scenarios. To this end, we functionalize resins with upconversion nanocrystals (UCNCs), namely an UCNC-Au composite structure, to endow them with the unique ability of converting near-infrared (NIR) radiation into visible-light emission. Such UCNC-functionalized resins with high transparency and flexibility are expected to accelerate the development in the comprehensive utilization of NIR during practical applications.