Bright Single-Photon Emitters with a CdSe Quantum Dot and Multimode Tapered Nanoantenna for the Visible Spectral Range

Nanomaterials (Basel). 2021 Apr 3;11(4):916. doi: 10.3390/nano11040916.

Abstract

We report on single photon emitters for the green-yellow spectral range, which comprise a CdSe/ZnSe quantum dot placed inside a semiconductor tapered nanocolumn acting as a multimode nanoantenna. Despite the presence of many optical modes inside, such a nanoantenna is able to collect the quantum dot radiation and ensure its effective output. We demonstrate periodic arrays of such emitters, which are fabricated by focused ion beam etching from a II-VI/III-V heterostructure grown using molecular beam epitaxy. With non-resonant optical pumping, the average count rate of emitted single photons exceeds 5 MHz with the second-order correlation function g(2)(0) = 0.25 at 220 K. Such single photon emitters are promising for secure free space optical communication lines.

Keywords: CdSe; MBE; nanoantenna; quantum dots; single-photon emission.