Interferometric Imaging of Solvent Vapor of Evaporating Liquid Films

Langmuir. 2021 May 4;37(17):5385-5392. doi: 10.1021/acs.langmuir.1c00566. Epub 2021 Apr 22.

Abstract

The liquid deposition of thin films requires a thorough understanding of the underlying drying process, as it is an essential subprocess, where many defects may arise. To complement experimental studies, the present study uses a laser Michelson interferometer to visualize the vapor cloud of evaporating liquid films. The recorded interferometric patterns are evaluated using windowed Fourier filtering and a novel phase-unwrapping algorithm to allow for a robust analysis. Thin solvent stripes of different lengths are combined to yield a quantitative two-dimensional distribution of the solvent vapor concentration along a thin liquid stripe. The results show a considerable influence of natural convection during evaporation.