Stretchable energy storage devices are essential for developing stretchable electronics and have thus attracted extensive attention in a variety of fields including wearable devices and bioelectronics. Carbon materials, e.g., carbon nanotube and graphene, are widely investigated as electrode materials for energy storage devices due to their large specific surface areas and combined remarkable electrical and electrochemical properties. They can also be effectively composited with many other functional materials or designed into different microstructures for fabricating stretchable energy storage devices. This review summarizes recent advances toward the development of carbon-material-based stretchable energy storage devices. An overview of common carbon materials' fundamental properties and general strategies to enable the stretchability of carbon-material-based electrodes are presented. The performances of the as-fabricated stretchable energy storage devices including supercapacitors, lithium-ion batteries, metal-air batteries, and other batteries are then carefully discussed. Challenges and perspectives in this emerging field are finally highlighted for future studies.
Keywords: carbon materials; lithium-ion batteries; metal-air batteries; stretchable supercapacitors.
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