Self-Motility of an Active Particle Induced by Correlations in the Surrounding Solution

Phys Rev Lett. 2020 Dec 31;125(26):268002. doi: 10.1103/PhysRevLett.125.268002.

Abstract

Current models of phoretic transport rely on molecular forces creating a "diffuse" particle-fluid interface. We investigate theoretically an alternative mechanism, in which a diffuse interface emerges solely due to a nonvanishing correlation length of the surrounding solution. This mechanism can drive self-motility of a chemically active particle. Numerical estimates indicate that the velocity can reach micrometers per second. The predicted phenomenology includes a bilinear dependence of the velocity on the activity and a possible double velocity reversal upon varying the correlation length.