Qualification of the activities measured by gamma spectrometry on unitary items of intermediate-level radioactive waste from particle accelerators

Patrycja Dyrcz; Thomas Frosio; Nabil Menaa; Matteo Magistris; Chris Theis

doi:10.1016/j.apradiso.2020.109431

Qualification of the activities measured by gamma spectrometry on unitary items of intermediate-level radioactive waste from particle accelerators

Appl Radiat Isot. 2021 Jan:167:109431. doi: 10.1016/j.apradiso.2020.109431. Epub 2020 Sep 22.

Authors

Patrycja Dyrcz¹, Thomas Frosio², Nabil Menaa³, Matteo Magistris³, Chris Theis³

Affiliations

¹ Radiation Protection Group, European Organization for Nuclear Research, 1211, Geneva 23, Switzerland. Electronic address: patrycja.kinga.dyrcz@cern.ch.
² Radiation Protection Group, European Organization for Nuclear Research, 1211, Geneva 23, Switzerland. Electronic address: thomas.frosio@gmail.com.
³ Radiation Protection Group, European Organization for Nuclear Research, 1211, Geneva 23, Switzerland.

PMID: 33011515
DOI: 10.1016/j.apradiso.2020.109431

Abstract

In the frame of maintenance, upgrade and dismantling activities, activated equipment are removed from the accelerator complex and require characterization in view of their disposal as radioactive waste. The characterization process consists of a series of radiation measurements, complemented by analytical studies, which quantify the activity of radionuclides inside an object. A fraction of the radioactive waste produced at CERN presents contact dose-rates higher than 100 μSv/h, and can therefore be classified as LILW Waste ("Low and intermediate level radioactive waste"). These objects, due to the activation mechanisms, are often subject to large activity heterogeneities. The quantification of gamma-emitting radionuclides is typically performed by gamma spectrometry, under the assumption of homogeneous distributions of activity within an object. However, this assumption can lead to underestimating the activity value of such radionuclides. In this article we perform a gamma spectrometry qualification in order to quantify the impact of assuming homogenous distribution.

Keywords: Gamma spectrometry qualification; Heterogeneous source matrix; Intermediate-level radioactive waste; Particle accelerators; Uncertainty quantification.